Phase diagrams: Effect of the potential range
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1 Phase diagrams: Effect of the potential range DLVO-potential: good qualitative agreement with the experiment experiment Effect on reentrance: simulation % 1,2 "# 1,2 $ 2" (! a = = # (! a ) Disks DLVO 1/r 12 1/r 6 Expt. Colloids! ! ! 1 /! s s 0 ) 1,2
2 Quanteneffekte für kleine Teilchenmassen?
3 Schema der effektiven Wechselwirkungen für N=3 und P=4: l = 3 J=1 l = 3 J=3 l = 4 l = 2 l = 4 l = 2 l = 1 l = 1 l = 4 l = 3 J=2 l = 1 l = 2
4 Zunahme des effektiven harte Kugel- Durchmessers aufgrund der Orts-Impuls Unschärfe: q.m. Δσ ~ Λ Τ / 2 3/2
5 Quantum effects on the phase diagram : Qualitative difference: quantum-melting (prediction!) qm : PIMC (P = 64) m * = mt" 2 =10.000
6 Colloidal dispersions: Strukturen im Gleichgewicht: Phasenumwandlungen und Quanteneffekte Strukturbildung im Nichtgleichgewicht Vergleich mit Experimenten und Voraussagen
7 Structure formation in two dimensions in confinement (walls) Layering and Lane Reduction: at defects L Study and analysis of structure formation mechanisms Effects of geometry (L), diameter ratios, composition, density, temperature, flow velocity, Comparison to three dimensional scenarios Test of thermodynamical approximations Mixtures:
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11 Method: Computer Simulations N particles in finite volume at temperature T (periodic boundary conditions / confinement) Molecular Dynamics Monte Carlo Brownian Dynamics Pair interactions: Repulsive interactions (magnetic)
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16 Recent cooperation with experimental projects (Erbe/Leiderer): M. Köppl, P. Henseler, A. Erbe, P. Nielaba, P. Leiderer, Phys. Rev. Lett. 97, (2006) Layer reduction in 2D model colloids in gravitational fields: 5 layers particle flow 4 layers Structure formation at walls in flow direction: Effect of external driving forces (F) in binary model colloids:
17 Das Universum im Computer / LS Nielaba Numerisch exakte Behandlung komplexer Systeme Überprüfung analytischer Näherungen Voraussagen fürs Experiment Vielteilchensysteme Quantenphänomene Magnetismus Materialien für die Zukunft Nano-Bauelemente Neue Speichermedien Struktur-Änderungen durch äußere Felder Nachbarwissenschaften: Mathematik (Modellbildung, Methoden), Informatik, Chemie (Moleküle), Biologie (Membran), Finanz-Physik ( )
18 Conductance (2e 2 /h) Electrode distance (nm) Quantization of the electrical conductance E.Scheer, physics department, University of Konstanz
19 Single-atom-contacts: Electronic properties of Nano-materials can differ much from those of macroscopic systems (example: conductance-quantization (AG Scheer) Questions: 1) Formation process of single atom contacts? 2) Current through these contacts? ad 1): MD-simulation of a stretching process in a Au-wire (M. Dreher) (Au-wire, 300 atoms, oriented in (100) direction) ad 2): Computation of current in these configurations Method: tight binding, thermal average (cooperation with C. Cuevas, J. Heurich and E. Scheer)
20 3 nm
21 Simulation of a stretched gold wire
22 Conductance-quantization in single-atom contacts: - Conductance-quantization in transport- channels due to the wave-nature of the electrons (see box-potential ):! G = I V = ev "n "E G = 2e 2 h [ ( )( µ 1 # µ 2 )T] ( µ 1 # µ 2 ) e N ( ) $ T i G 0 = ( 2e 2 /h) i=1 ( ) T [ ] = 2e 2 h (one channel) (N channels) (Landauer-Büttiker-formalism, PRB31,6207 (85)) - Computation of G in tight-binding - approximation: H = ' i#,$ G = 2e h + " i# c i#,$ c i#,$ + ( ) Tr ˆ ' i#& j%,$ + t i#,j% c i#,$ c j%,$ ( t t ˆ + ), t ˆ t ˆ + ( Matrix with N Eigen values T i, G = G 0 ' T i (Levy Yeyati et al., PRB56, (97), Cuevas et al., PRL80, 1066 (98)) N i=1
23 experimental : values (E. Scheer)
24 Aus: A.I. Yanson, Atomic chains and electronic shells: quantum mechanisms for the formation of nanowires Ph.D. thesis, Leiden (2001).
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26 Das Universum im Computer / LS Nielaba Numerisch exakte Behandlung komplexer Systeme Überprüfung analytischer Näherungen Voraussagen fürs Experiment Vielteilchensysteme Quantenphänomene Magnetismus Materialien für die Zukunft Nano-Bauelemente Neue Speichermedien Struktur-Änderungen durch äußere Felder Nachbarwissenschaften: Mathematik (Modellbildung, Methoden), Informatik, Chemie (Moleküle), Biologie (Membran), Finanz-Physik ( )
27 References: Phys. Rev. E78, (2008) Phys. Rev. E76, (2007) Phys. Rev. E76, (2007) Phys. Rev. E75, (2007) Phys. Rev. Lett. 97, (2006) Phys. Rev. B74, (2006) Phys. Rev. B72, (2005) Phys. Rev. Lett. 90, (2003) Phys. Rev. E66, (2002) Phys. Rev. E63, (2001)
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